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There aren't all that many 'song dubbed over a still photo' clips that I'll five-star automatically, but pretty much anything by the Sonics is in the running.
I just came here to submit this, beaten, but here's a version with some appropriate psycho-a-go-go video: http://www.youtube.com/watch?v=Dw6Fjo6VXTg
The Sonics.
I like "Strychnine" or "The Witch" better but still: The Sonics.
One of the pinnacles of civilisation!